Synthesis of diarylmethylamines via palladium-catalyzed regioselective arylation of 1,1,3-triaryl-2-azaallyl anions

Minyan Li, Baris Yücel, Javier Adrio, Ana Bellomo, Patrick J. Walsh*

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85 Atıf (Scopus)

Özet

Diarylmethylamines are of great interest due to their prevalence in pharmaceutical chemistry. As a result, new methods for their synthesis are in demand. Herein, we report a versatile protocol for the synthesis of diarylmethylamine derivatives involving palladium-catalyzed arylation of in situ generated 2-azaallyl anion intermediates. The 2-azaallyl anions are generated by reversible deprotonation of readily available aldimine and ketimine precursors. Importantly, the arylated aldimine and ketimine products do not undergo isomerization under the reaction conditions. Scale-up of the arylation and hydrolysis of the resulting products to furnish diarylmethylamines were also successfully performed. This journal is

Orijinal dilİngilizce
Sayfa (başlangıç-bitiş)2383-2391
Sayfa sayısı9
DergiChemical Science
Hacim5
Basın numarası6
DOI'lar
Yayın durumuYayınlandı - Haz 2014

Finansman

FinansörlerFinansör numarası
National Institute of General Medical Sciences104349
National Institutes of Health
National Stroke FoundationCHE-1152488

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