TY - JOUR
T1 - Neutron and gamma-ray shielding effectiveness of novel polyaniline composites
AU - Kahraman, Deniz Agehan
AU - Cogalmis, Fatma Tuba
AU - Esen, Ayse Nur
AU - Haciyakupoglu, Sevilay
AU - Senkal, Bahire Filiz
N1 - Publisher Copyright:
© 2024 Elsevier Ltd
PY - 2024/6
Y1 - 2024/6
N2 - This study uses experimental, theoretical, and Monte Carlo simulation techniques to investigate the neutron and gamma-ray shielding performances of polyaniline-based composites filled with different amounts of formic acid, boron nitride, and boric acid. The radiation shielding performances of composites were evaluated at neutron energies of 0.025 eV, 1 keV, and 10 MeV, and gamma-ray energy of 662 keV. The study found that the composite material made of polyaniline and boron nitride with a higher percentage of boron has better thermal neutron shielding properties than other polyaniline composites. The research also showed that a polyaniline-boric acid composite with a thickness of 1.6 mm can reduce thermal neutrons by 64.5%. As a result, the composite containing equal amounts of polyaniline and boric acid was identified as the most promising material for shielding. The macroscopic cross-sections of neutrons and mass attenuation coefficients of gamma-rays were found to have expanded uncertainties up to 13.47% and 7.11%, respectively. The factors contributing to the uncertainty of the experimental, theoretical, and simulation results were identified, evaluated, and shown how to include uncertainty components in the uncertainty budget.
AB - This study uses experimental, theoretical, and Monte Carlo simulation techniques to investigate the neutron and gamma-ray shielding performances of polyaniline-based composites filled with different amounts of formic acid, boron nitride, and boric acid. The radiation shielding performances of composites were evaluated at neutron energies of 0.025 eV, 1 keV, and 10 MeV, and gamma-ray energy of 662 keV. The study found that the composite material made of polyaniline and boron nitride with a higher percentage of boron has better thermal neutron shielding properties than other polyaniline composites. The research also showed that a polyaniline-boric acid composite with a thickness of 1.6 mm can reduce thermal neutrons by 64.5%. As a result, the composite containing equal amounts of polyaniline and boric acid was identified as the most promising material for shielding. The macroscopic cross-sections of neutrons and mass attenuation coefficients of gamma-rays were found to have expanded uncertainties up to 13.47% and 7.11%, respectively. The factors contributing to the uncertainty of the experimental, theoretical, and simulation results were identified, evaluated, and shown how to include uncertainty components in the uncertainty budget.
KW - Composite
KW - Gamma-ray
KW - Geant4
KW - Neutron
KW - Polyaniline
KW - Shielding
UR - http://www.scopus.com/inward/record.url?scp=85188508797&partnerID=8YFLogxK
U2 - 10.1016/j.radphyschem.2024.111675
DO - 10.1016/j.radphyschem.2024.111675
M3 - Article
AN - SCOPUS:85188508797
SN - 0969-806X
VL - 219
JO - Radiation Physics and Chemistry
JF - Radiation Physics and Chemistry
M1 - 111675
ER -