Transformation of 2,4-dichlorophenol by H 2O 2/UV-C, Fenton and photo-Fenton processes: Oxidation products and toxicity evolution

Akin Karci, Idil Arslan-Alaton*, Tugba Olmez-Hanci, Miray Bekbölet

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

112 Citations (Scopus)

Abstract

In the present study, H 2O 2/UV-C, Fenton and photo-Fenton treatment of 2,4-dichlorophenol was compared in terms of oxidation products and acute toxicity. The oxidation products were identified by gas chromatography-mass spectroscopy, high performance liquid chromatography and ion chromatography, whereas changes in acute toxicity were evaluated by the Vibrio fischeri luminescence inhibition assay. H 2O 2/UV-C and photo-Fenton processes ensured complete 2,4-dichlorophenolremoval, detoxification and significant mineralization. Hydroquinone and formic acid were identified as the common oxidation products of the studied advanced oxidation processes investigated. 3,5-dichloro-2-hydroxybenzaldehyde, phenol, 4-chlorophenol and 2,5-dichlorohydroquinone were identified as the additional H 2O 2/UV-C oxidation products of 2,4-dichlorophenol. Acute toxicity decreased with decreasing 2,4-dichlorophenol and increasing chloride release.

Original languageEnglish
Pages (from-to)65-73
Number of pages9
JournalJournal of Photochemistry and Photobiology A: Chemistry
Volume230
Issue number1
DOIs
Publication statusPublished - 15 Feb 2012

Funding

The financial support of the Scientific and Technological Research Council of Turkey (TUBITAK, Project No: 111Y145) is gratefully acknowledged. The study was conducted at the laboratory facilities of Istanbul Technical University, Environmental Engineering Department.

FundersFunder number
TUBITAK111Y145
Türkiye Bilimsel ve Teknolojik Araştirma Kurumu

    Keywords

    • 2,4-Dichlorophenol (2,4 DCP)
    • Acutetoxicity
    • Fenton
    • H O /UV-C
    • Oxidation product
    • Photo-Fenton

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