High capacity and high density functional conductive polymer and SiO anode for high-energy lithium-ion batteries

Hui Zhao; Neslihan Yuca; Ziyan Zheng; Yanbao Fu; Vincent S. Battaglia; Guerfi Abdelbast; Karim Zaghib; Gao Liu

doi:10.1021/am507376f

High capacity and high density functional conductive polymer and SiO anode for high-energy lithium-ion batteries

Hui Zhao, Neslihan Yuca, Ziyan Zheng, Yanbao Fu, Vincent S. Battaglia, Guerfi Abdelbast, Karim Zaghib, Gao Liu^*

^*Corresponding author for this work

Energy Institute

Research output: Contribution to journal › Article › peer-review

73 Citations (Scopus)

Abstract

High capacity and high density functional conductive polymer binder/SiO electrodes are fabricated and calendered to various porosities. The effect of calendering is investigated in the reduction of thickness and porosity, as well as the increase of density. SiO particle size remains unchanged after calendering. When compressed to an appropriate density, an improved cycling performance and increased energy density are shown compared to the uncalendered electrode and overcalendered electrode. The calendered electrode has a high-density of ∼1.2 g/cm³. A high loading electrode with an areal capacity of ∼3.5 mAh/cm² at a C/10 rate is achieved using functional conductive polymer binder and simple and effective calendering method.

Original language	English
Pages (from-to)	862-866
Number of pages	5
Journal	ACS applied materials & interfaces
Volume	7
Issue number	1
DOIs	https://doi.org/10.1021/am507376f
Publication status	Published - 14 Jan 2015

Bibliographical note

Publisher Copyright:
© 2014 American Chemical Society.

Funding

Funders	Funder number
U.S. Department of Energy	#DE-AC02-05CH11231

Keywords

calendering
conductive polymer binder
lithium-ion battery
silicon monoxide

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1021/am507376f

Cite this

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abstract = "High capacity and high density functional conductive polymer binder/SiO electrodes are fabricated and calendered to various porosities. The effect of calendering is investigated in the reduction of thickness and porosity, as well as the increase of density. SiO particle size remains unchanged after calendering. When compressed to an appropriate density, an improved cycling performance and increased energy density are shown compared to the uncalendered electrode and overcalendered electrode. The calendered electrode has a high-density of ∼1.2 g/cm3. A high loading electrode with an areal capacity of ∼3.5 mAh/cm2 at a C/10 rate is achieved using functional conductive polymer binder and simple and effective calendering method.",

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AU - Zhao, Hui

AU - Yuca, Neslihan

AU - Zheng, Ziyan

AU - Fu, Yanbao

AU - Battaglia, Vincent S.

AU - Abdelbast, Guerfi

AU - Zaghib, Karim

AU - Liu, Gao

PY - 2015/1/14

Y1 - 2015/1/14

N2 - High capacity and high density functional conductive polymer binder/SiO electrodes are fabricated and calendered to various porosities. The effect of calendering is investigated in the reduction of thickness and porosity, as well as the increase of density. SiO particle size remains unchanged after calendering. When compressed to an appropriate density, an improved cycling performance and increased energy density are shown compared to the uncalendered electrode and overcalendered electrode. The calendered electrode has a high-density of ∼1.2 g/cm3. A high loading electrode with an areal capacity of ∼3.5 mAh/cm2 at a C/10 rate is achieved using functional conductive polymer binder and simple and effective calendering method.

AB - High capacity and high density functional conductive polymer binder/SiO electrodes are fabricated and calendered to various porosities. The effect of calendering is investigated in the reduction of thickness and porosity, as well as the increase of density. SiO particle size remains unchanged after calendering. When compressed to an appropriate density, an improved cycling performance and increased energy density are shown compared to the uncalendered electrode and overcalendered electrode. The calendered electrode has a high-density of ∼1.2 g/cm3. A high loading electrode with an areal capacity of ∼3.5 mAh/cm2 at a C/10 rate is achieved using functional conductive polymer binder and simple and effective calendering method.

KW - calendering

KW - conductive polymer binder

KW - lithium-ion battery

KW - silicon monoxide

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High capacity and high density functional conductive polymer and SiO anode for high-energy lithium-ion batteries

Abstract

Bibliographical note

Funding

Keywords

UN SDGs

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