A Tripartite Composite Incorporating Nitrogen-Doped Graphene Oxide, Polypyrrole, and Silica for Lithium-Ion Battery Anodes

Mohammed Al-Bujasim, Metin Gencten*, Koray B. Donmez, Melih B. Arvas, Nilgun Karatepe, Yucel Sahin

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

In this study, N-doped graphene oxide-polypyrrole-silica (NGO-PPy-SiO2) composite was employed as a possible anode in Li-ion batteries. The chronoamperometric technique was employed to synthesize NGO, and within this study two samples were produced, one characterized by a high polypyrrle content (N1) and the other by a low polypyrrle content (N2). N2 has the maximum initial discharge capacity of 785 mAh g−1 at 0.1 C, which is greater than N1’s capacity of 501 mAh g−1. The initial coulombic efficiency of the first cycle is around 72%, whereas the ICE of N2 is approximately 60%. N1 demonstrates outstanding cycling performance for 100 cycles at high rate (10 C) with maintain capacity as 100% and coulombic efficiency of 100%, as well as extremely stable capacity during the cycling. N2 has a maintain capacity of ≈79% and excellent coulombic efficiency, however the capacity during cycling is not as stable as N1.

Original languageEnglish
Article number051001
JournalECS Journal of Solid State Science and Technology
Volume13
Issue number5
DOIs
Publication statusPublished - May 2024

Bibliographical note

Publisher Copyright:
© 2024 The Electrochemical Society (“ECS”). Published on behalf of ECS by IOP Publishing Limited.

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